By Guy P. Brasseur, Susan Solomon
"[…] an enticing and well-written evaluation of the present prestige of our wisdom of the composition of the center surroundings and the elemental radiative, dynamical and photochemical techniques which hold it." (Bulletin American Meteorological Society)
Read Online or Download Aeronomy of the Middle Atmosphere: Chemistry and Physics of the Stratosphere and Mesosphere (Atmospheric and Oceanographic Sciences Library) PDF
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Extra info for Aeronomy of the Middle Atmosphere: Chemistry and Physics of the Stratosphere and Mesosphere (Atmospheric and Oceanographic Sciences Library)
This is not always the case, since B and C may also be undergoing production and destruction reactions that introduce a time dependence in their densities over the time τA . In a system like the atmosphere, in which numerous gases are interacting simultaneously, chemical change usually occurs through a network of interacting steps (reaction mechanism). 38) (A) = k1 (B) + k2 (C)(M) + k3 (F) In some cases, the eﬀective rate of a reaction can be increased by a so-called catalytic cycle of intermediate reactions.
1) and radiative decay can occur. 2) The selection rules for radiative processes permit us to evaluate the ease or diﬃculty with which a particular transition can proceed. The basic rules are as follows: ∗ Spin is unchanged in an allowed transition, for both atoms and molecules. This is generally the most important consideration in establishing the transition probability. ∗ L or Λ changes of 1 or zero are allowed, except in the case of atoms if 0 → 0 (S → S). , D → S) are unfavorable. ∗ For molecules with g and u subscripts, g → u transitions are allowed, but u → u or g → g transitions are diﬃcult.
The rate at which a chemical reaction occurs varies considerably from one reaction to another and must be determined in the laboratory. For a reaction between species A, B, C, . , expressed as aA + bB + cC + . . → mM + nN + . . 21) where coeﬃcients a, b, c, etc. are the smallest possible integers that provide the correct stoichiometry, the reaction rate R can be expressed by the general expression R = f [(A), (B), (C), . . 22) where (A) represents the concentration of species A. As shown by experimental studies, this function may be complex, but may often be of the form R = k(A)α (B)β (C)γ .
Aeronomy of the Middle Atmosphere: Chemistry and Physics of the Stratosphere and Mesosphere (Atmospheric and Oceanographic Sciences Library) by Guy P. Brasseur, Susan Solomon